Export citation

Export citation

Choose format for download:

Download Citation

    Emergence of Long-Ranged Stress Correlations at the Liquid to Glass Transition

    Manuel Maier1, Annette Zippelius2, and Matthias Fuchs1

    • 1University of Konstanz, D-78457 Konstanz, Germany
    • 2University Göttingen, D-37077 Göttingen, Germany

    Phys. Rev. Lett. 119, 265701 – Published 29 December, 2017

    DOI: https://doi.org/10.1103/PhysRevLett.119.265701

    Abstract

    A theory for the nonlocal shear stress correlations in supercooled liquids is derived from first principles. It captures the crossover from viscous to elastic dynamics at an idealized liquid to glass transition and explains the emergence of long-ranged stress correlations in glass, as expected from classical continuum elasticity. The long-ranged stress correlations can be traced to the coupling of shear stress to transverse momentum, which is ignored in the classic Maxwell model. To rescue this widely used model, we suggest a generalization in terms of a single relaxation time τ for the fast degrees of freedom only. This generalized Maxwell model implies a divergent correlation length ξ∝τ as well as dynamic critical scaling and correctly accounts for the far-field stress correlations. It can be rephrased in terms of generalized hydrodynamic equations, which naturally couple stress and momentum and furthermore allow us to connect to fluidity and elastoplastic models.

    Physics Subject Headings (PhySH)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    Supplemental Material (Subscription Required)

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation